IR Spectra of Dye Molecules Calculated Using Density Functional Theory

Abstract

Calculations of IR absorption spectra for energy-minimized dye molecules using density function theory (DFT) are presented. These calculations can provide interpretation of absorption spectra with respect to isolated molecular structure for excitation by electromagnetic waves at IR frequencies. The absorption spectra corresponding to excitation states of isolated molecules are to be associated with molecular-level response modes that are uncoupled to other molecules at zero temperature, in contrast to that of bulk systems at finite temperature. DFT-calculated absorption spectra represent quantitative estimates that can be correlated with additional information obtained from laboratory measurements. The DFT software GAUSSIAN was used for calculations of vibrational excitation states presented here.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Nov 21, 2019
Accession Number
AD1086070

Entities

People

  • Andrew Shabaev
  • Lulu Huang
  • Samuel G. Lambrakos

Organizations

  • United States Naval Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Absorption
  • Absorption Spectra
  • Cartesian Coordinates
  • Charge Density
  • Density Functional Theory
  • Department Of Defense
  • Energy
  • Frequency
  • Geometry
  • Ground State
  • Intensity
  • Materials
  • Materials Science
  • Military Research
  • Molecules
  • Optimization
  • Spectra

Fields of Study

  • Physics

Readers

  • Chemistry (specifically Chemical Fluorescence)
  • Quantum Chemistry