Single Step Bonding of Thick Anodized Aluminum Oxide Templates to Silicon Wafers for Enhances System-on-a-Chip Performance

Abstract

Vertically-aligned nanowires are of interest for novel applications including sensing, photonics, and energy storage. Templated synthesis of such structures has been previously demonstrated via anodized aluminum oxide (AAO). However, the performance of AAO-on-Si devices has been limited by current methods of obtaining well-adhered, thick AAO templates on Si substrates. Thicker AAO templates allow for longer nanowires of active material, which is expected to increase performance of devices reliant on the surface area or volume of the active material. In this report, Al-Si eutectic bonding was used to achieve thick AAO-on-Si, with templates up to 90 m thick bonded to the wafer. Carbon nanotubes (CNTs) were grown in the AAO templates bonded to Si to create proof-of-concept on-chip supercapacitor devices. Our devices show a promising value of 0.44 mF cm-2, much higher than previous AAO-on-Si capacitors. The structure of the CNT/AAO/Si stack is examined using SEM and TEM, and the device performance is tested through cyclic voltammetry (CV), electrochemical impedance spectroscopy (EIS), and galvanostatic charge-discharge (GCD) measurements.

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Document Details

Document Type
Technical Report
Publication Date
Jan 15, 2020
Accession Number
AD1090823

Entities

People

  • Gibson P. Scisco
  • Katherine Haynes
  • Kevin S. Jones
  • Kirk J Ziegler

Organizations

  • University of Florida

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Air Force
  • Aluminum
  • Aluminum Oxides
  • Capacitance
  • Capacitors
  • Carbon Nanotubes
  • Chemical Vapor Deposition
  • Chemistry
  • Electrochemical Capacitors
  • Energy Storage
  • Films
  • Fullerenes
  • Heat Treatment
  • Materials
  • Materials Processing
  • Materials Science
  • Supercapacitors

Fields of Study

  • Materials science

Readers

  • Electrochemical Surface Science
  • Nanocomposite Materials Science
  • Surface Engineering/Surface Coating Technology.