Improved Ceramic Manufacturability With Electric Field Assisted Sintering: Developing Underlying Principles

Abstract

High density ceramics maximize strength, translucency, thermal conductivity and provide gas tight environments. These features are key to applications ranging from armor, IR missile domes, integrated circuit substrates and solid oxide fuel cell electrolytes, respectively. To achieve desired high densities for such highly refractory materials, sintering (at times requiring hot isostatic pressing) must be performed at temperatures often in excess of 1500 deg C for extended periods of time, leading to high costs, need for specialized facilities and incompatibility with less refractory materials. While conventional densification methods utilizing high temperature and pressure have reached their limits, electric field assisted sintering has demonstrated great potential in reducing temperature constraints imposed on ceramic materials during sintering. Application of electrical fields during sintering can reduce densification temperatures from above 1300 deg C to 800 deg C, to times as short as seconds, the latter via Flash Sintering (FS). While there have been many phenomenological observations and demonstrations of Field Assisted Sintering (FAST), reliable micro and nanoscale descriptions remain lacking (1). This is not surprising given that the electrical and mass transport properties of ceramic materials differ so widely, ranging from highly insulating to metallic, from predominantly ionic to electronic conductors and all with properties highly dependent on microstructure.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Mar 29, 2020
Accession Number
AD1097893

Entities

People

  • Bilge Yıldız
  • Harry L Tuller

Organizations

  • Massachusetts Institute of Technology

Tags

Communities of Interest

  • Advanced Electronics
  • Biomedical
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Ceramic Materials
  • Chemistry
  • Electric Fields
  • Electrical Properties
  • Electrons
  • Energy
  • Engineering
  • Fuel Cells
  • Geometry
  • High Temperature
  • Materials
  • Materials Science
  • Measurement
  • Partial Pressure
  • Refractory Materials
  • Space Charge
  • Transport Properties

Fields of Study

  • Materials science

Readers

  • Reinforced Composite Materials
  • Surface Engineering/Surface Coating Technology.
  • Systems Analysis and Design

Technology Areas

  • Biotechnology
  • Microelectronics