Spectroscopic and Electrochemical Studies of Transition-Metal Tetrasulfonated Phthalocyanines. VI. The Adsorption of Iron Tetrasulfonated Phthalocyanine on Single Crystal Silver Electrodes.

Abstract

Adsorbed layers of iron tetrasulfonated phthalocyanine have been examined using cyclic voltammetry on the silver single crystal low index surface: (100), (110), and (111). The peak potentials and charge under the voltammetry peaks show some dependence on the crystal planes. The effects of the underpotential deposition of lead on the adsorbed macrocycle have also been examined on the silver single crystal electrode. The lead can be underpotential deposited on the silver directly through a pre-adsorbed macrocycle layer without desorbing the macrocycle. The data are explained in terms of a model for the adsorbed macrocycle which has the plane of the ligand perpendicular to the electrode surface.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Nov 01, 1985
Accession Number
ADA161640

Entities

People

  • B. Simic-glavaski
  • E. B. Yeager
  • R. Adzic

Organizations

  • Case Western Reserve University

Tags

Communities of Interest

  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Charge Transfer
  • Chemistry
  • Crystal Structure
  • Crystals
  • Desorption
  • Electrochemical Cells
  • Electrochemistry
  • Electrodes
  • Metals
  • Military Research
  • Raman Spectroscopy
  • Single Crystals
  • Spectra
  • Standards
  • Transition Metals
  • Transitions
  • United States

Fields of Study

  • Chemistry

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Electrochemical Surface Science
  • Materials Science and Engineering.