Characterization of Substituted Phenol-Formaldehyde Resins Using Solid-State Carbon-13 NMR

Abstract

Crosslinked substituted phenol-formaldehyde resins were synthesized from cashew nut shell liquid, 3-n-pentadecylphenol and phenol with formaldehyde. The resulting resins were crosslinked and then investigated using carbon-13 NMR in the solid state using cross-polarization, magic angle spinning, and dipolar decoupling. Comparisons were made between the spectra of pure phenol-formaldehyde and modified phenol-formaldehyde resins and it was shown possible to distinguish between the resins. It was also shown that the proton-dephased spectrum gave better spectral resolution for the substituted compounds. In addition, the solids carbon-13 technique verified that the degradation of the substituted phenolic resins occurs first with the degradation of the side chain in agreement with suggestions from earlier work.

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Document Details

Document Type
Technical Report
Publication Date
Jul 30, 1988
Accession Number
ADA208744

Entities

People

  • Brijnaresh R. Sinha
  • Daniel T. O'Connor
  • Frank D. Blum

Tags

Communities of Interest

  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Agreements
  • Aldehydes
  • Chemical Shifts
  • Chemical Synthesis
  • Chemistry
  • Cross Polarization
  • Decoupling
  • Degradation
  • Formaldehyde
  • High Temperature
  • Materials
  • Military Research
  • Missouri
  • Organic Chemistry
  • Resonance
  • Spectra
  • Thermal Stability

Fields of Study

  • Materials science

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  • Organic Chemistry
  • Solar Physics