Use of Time-Dependent Chemical Sensor Signals for Selective Identification

Abstract

A sensor is described for identifying and quantifying different components in a gas mixture by decoding information from a modulated output signal. The system operates by passing the unknown gas into a reaction chamber containing a heated catalytic filament. The output products of the chamber are detected by an electrochemical sensor. The concentration of the reaction products is modulated by varying the temperature of the catalytic filament. A theory is presented for analyzing the modulated output signal. The validity of the analysis is confirmed by experiments conducted with benzene, Carbon Monoxide, Hydrogen Cyanide, and by computer simulations. It appears possible to identify different species in the inlet gas stream if the species undergo chemical reactions in the reactor that have different activation energies. The signal magnitude at peaks or valleys in the output is directly proportional to concentrations even though a steady-state condition is not reached. The approach may be generalized to other detector systems. Keywords: Microsensors, Time dependent sensor, Electrochemical sensor, Activation energy.

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Document Details

Document Type
Technical Report
Publication Date
Jun 01, 1989
Accession Number
ADA212729

Entities

People

  • G. J. Maclay
  • Joseph R. Stetter
  • Steven D. Christesen

Organizations

  • Edgewood Chemical Biological Center

Tags

Communities of Interest

  • Materials and Manufacturing Processes
  • Sensors

DTIC Thesaurus Topics

  • Arrhenius Equation
  • Chemical Analysis
  • Chemical Detectors
  • Chemical Reaction Properties
  • Chemical Reactions
  • Chemistry
  • Computer Simulations
  • Detection
  • Detectors
  • Electrochemical Cells
  • Energy
  • Engineering
  • Heat Of Activation
  • Measurement
  • Simulations
  • Steady State
  • Warning Systems

Readers

  • Combustion and Flow Dynamics.
  • Organic Chemistry
  • Radio communications and signal processing.