Azo Polymers for Reversible Optical Storage.11. Poly(4,4'-(1- Methylidene)Bisphenylene-3-4-(4-Nitrophenylazo)Phenyl3-Aza-Pentanedionate).

Abstract

Poly(4,4'-(1-methylethylidene)bisphenylene 3-(4-(4-nitrophenylazo)phenyl-3-aza-pentanedioate! (pMNAP) was synthesized through the condensation polymerization of 4,4'-isopropylidene-bis-phenol and N-4-(4-NITROPHENYLAZO)PHENYLimido diacetyl chloride. The polymer solution in tetrahydrofuran (THF) was spin-coated onto a glass substrate to form a film and the process of reversibly photoinduced birefringence was tested. The birefringence induced in the film was observed at a level of 0.04. The biexponential fitting of the birefringence growth and relaxation curves shows two kinds of processes. A fairly low birefringence relaxation occurs after the light is turned off, about 12% at room temperature and less than 50% at 138 deg C, close to the glass transition temperature (152 deg C). pMNAP decomposes at about 160 deg C which prevents its use as a material for optical storage.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Mar 28, 1996
Accession Number
ADA306626

Entities

People

  • Almeria L. Natansohn
  • Paula A. Rochon
  • Xianghai Meng

Organizations

  • Queen's University

Tags

Communities of Interest

  • Air Platforms

DTIC Thesaurus Topics

  • Alkenes
  • Chemical Synthesis
  • Chemistry
  • Chlorides
  • Films
  • Glass
  • Glass Transition Temperature
  • Laser Beams
  • Macromolecules
  • Materials
  • Optical Storage
  • Polyesters
  • Polymeric Films
  • Polymers
  • Reversible
  • Transition Temperature
  • Transitions

Fields of Study

  • Chemistry

Readers

  • Polymer Science and Technology