Quantitative Analysis of the Detection Limits for Heavy Metal-Contaminated Soils by Laser-Induced Breakdown Spectroscopy

Abstract

Laser-induced breakdown spectroscopy (LIBS) is a rapid remote measurement method for detection of metals in the environment. A major factor in the quantitative use of this technique involves the minimum detection limits under both laboratory and field operations. Research on limits of detection of heavy metals in different types of soils under various conditions using LIBS has been carried out under Contract DACA39-95-K-0053. Pulses from a Nd:YAG laser operating at 125 mJ at lambda = 1.06 micrometers are focused on sample surfaces to produce laser sparks (plasmas). Atomic emissions from the plasmas are recorded using an optical multichannel analyzer after delays of a few microseconds when interference from broad-band emissions is reduced. Research has been performed on the detection limits of arsenic, cadmium, chromium, mercury, lead, and zinc in soil matrices. Results are reported on the lower detection limits of these six elements in sand, silt, clay, and kaolin matrices. Detection limits are significantly lower for heavy metals in sand matrices than silt and clay matrices due to differences between surface and volume contamination.

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Document Details

Document Type
Technical Report
Publication Date
Jun 01, 1997
Accession Number
ADA328435

Entities

People

  • Dana E. Poulain
  • Dennis R. Alexander

Organizations

  • University of Nebraska–Lincoln

Tags

Communities of Interest

  • Advanced Electronics
  • Sensors

DTIC Thesaurus Topics

  • Army Corps Of Engineers
  • Contamination
  • Detection
  • Detectors
  • Elements
  • Emission Spectra
  • Heavy Metals
  • Laser Spectroscopy
  • Laser-Induced Breakdown Spectroscopy
  • Lasers
  • Measurement
  • Metals
  • Nebraska
  • Research Facilities
  • Spectra
  • Spectroscopy
  • United States

Fields of Study

  • Physics

Readers

  • Groundwater Contamination Remediation.
  • Pulsed Power and Plasma Physics.
  • Surface Coatings Technology.

Technology Areas

  • Directed Energy