Growth of Low Defect Density Gallium Nitride (GaN) Films on Novel Tantalum Carbide (TaC) Substrates for Improved Device Performance

Abstract

To potentially improve device performance, we attempted to grow gallium nitride (GaN) films with better crystalline quality (fewer mismatch dislocations) using a tantalum carbide (TaC) substrate, which is more closely lattice matched to GaN than currently used substrates. We created the TaC substrate, using pulse laser deposition (PLD) of TaC onto (0001) SiC substrates at tilde 1000 deg C, and grew GaN films, using metal organic chemical vapor deposition (MOCVD). Using x-ray diffraction, we determined the TaC films grown on-axis were higher quality than the off-axis films, but the latter could be improved to a comparable quality by annealing at 1200-1600 deg C for 30 min. We also deposited GaN films onto the TaC after it had been nitrided with NH3 for 3 min at 1100 deg C and used aluminum nitride (AlN) as a low temperature nucleation layer. Using these methods, the crystalline quality of the GaN films was higher - the grains were tilde 10 times larger than those typically seen in films grown on SiC or sapphire, and they contained more than an order of magnitude fewer dislocations compared to a typical value of 4 x 10(exp 9) sq cm. However, the grains lacked the required (0001) texture, producing a very rough surface.

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Document Details

Document Type
Technical Report
Publication Date
May 01, 2009
Accession Number
ADA499547

Entities

People

  • K. A. Jones
  • K. W. Kirchner
  • M. A. Derenge
  • R. D. Vispute
  • T. S. Zheleva

Organizations

  • United States Army Research Laboratory

Tags

Communities of Interest

  • Advanced Electronics
  • Air Platforms
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Aluminum Nitrides
  • Ceramic Materials
  • Chemical Vapor Deposition
  • Compound Semiconductors
  • Crystal Structure
  • Crystals
  • Diffraction
  • Electron Microscopy
  • Gallium Nitrides
  • Metal-Semiconductor Junctions
  • Nitrides
  • Phase Diagrams
  • Silicon Carbide
  • Tantalum Carbides
  • Vapor Deposition
  • X Rays
  • X-Ray Diffraction

Fields of Study

  • Materials science

Readers

  • Powder metallurgy of Titanium alloys.
  • Semiconductor Device Technology
  • Thin Film Deposition Science.

Technology Areas

  • Directed Energy
  • Directed Energy - Pulsed-Laser Deposition
  • Microelectronics
  • Microelectronics - Graphene