Plasma-Enhanced Chemical Vapor Deposition of SiOx Films Using Electron Beam Generated Plasmas

Abstract

Tetraethyl orthosilicate (TEOS) was used as a silicon source to grow SiO2 films in a modulated electron beam generated plasma enhanced chemical vapor deposition (PECVD) arrangement. Process parameters investigated were: substrate temperature, gas composition, duty factor, and incident ion energy. At high temperatures (>150 C), film compositions were less sensitive to the process parameters, while at lower temperatures, the film chemistries varied greatly. Activation energies of -0.122 eV and -0.020 eV were determined for the films grown in these respective temperature ranges. Below 250 C, preferred growth conditions (> 20 nm/min) were found at small flow percentages of TEOS in argon/oxygen mixtures (2:48:50) with increased ion energies. The trade-off between substrate temperature and incident ion energy demonstrated a process viability not previously seen in scalable PECVD systems.

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Document Details

Document Type
Technical Report
Publication Date
Sep 28, 2009
Accession Number
ADA507111

Entities

People

  • Darrin Leonhardt
  • Ronald T. Holm
  • Scott G. Walton

Organizations

  • United States Naval Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Chemical Reaction Properties
  • Chemical Reactions
  • Chemical Vapor Deposition
  • Chemistry
  • Dissociation
  • Electrical Properties
  • Ionization
  • Low Temperature
  • Mass Spectra
  • Mass Spectrometers
  • Materials
  • Measurement
  • Physical Vapor Deposition
  • Power Electronics
  • Refractive Index
  • Silicon Dioxide
  • Vapor Deposition

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.
  • Pulsed Power and Plasma Physics.
  • Thin Film Deposition Science.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers
  • Directed Energy - Pulsed-Laser Deposition
  • Microelectronics
  • Microelectronics - Graphene