Kinetic Studies of Nonequilibrium Plasma-Assisted Combustion

Abstract

This project focuses on an integrated experimental/modeling study of hydrocarbon oxidation mechanisms under conditions of extreme thermal non-equilibrium. Large, and highly nonequilibrium, initial pools of important hydrocarbon combustion intermediate and electronically excited air species are created in a short pulsed fuel-air plasmas, created using approx 10-20 nsec duration - high (approx 20 kV) voltage pulsers, capable of operation at repetition rates as high as 40-50 kHz. The time evolution of critical species and temperature, after application of a single nanosecond discharge pulse, or a rapid "burst" of pulses, depending upon the experiment, are experimentally determined using advanced laser-based optical diagnostic methods. Results are compared to theoretical predictions from discharge and plasma chemical kinetic codes, developed as part of this program, in order to provide model validation and to improve understanding of fundamental nonequilibrium plasma kinetics in air and air/fuel mixtures.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Feb 25, 2010
Accession Number
ADA524301

Entities

People

  • Igor V. Adamovich
  • Walter R. Lempert

Organizations

  • Ohio State University

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies
  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Chemical Reaction Properties
  • Chemistry
  • Combustion
  • Dynamics
  • Fluid Dynamics
  • Hydrocarbons
  • Ignition
  • Kinetics
  • Laser Induced Fluorescence
  • Low Temperature
  • Measurement
  • Mechanical Engineering
  • Physics
  • Propulsion Systems
  • Raman Spectroscopy
  • Repetition Rate
  • Voltage

Fields of Study

  • Physics

Readers

  • Combustion science or combustion engineering.
  • Computational Modeling and Simulation
  • Electrical Engineering

Technology Areas

  • Directed Energy
  • Microelectronics