Experimental and Numerical Characterization of Polymer Nanocomposites for Solid Rocket Motor Internal Insulation

Abstract

The objective of this research is to develop a modeling framework for simulating the insulative behavior of thermoplastic Polyurethane elastomer nanocomposites (TPUNs) for solid rocket motors (SRMs) and the creation of software capable of predicting the properties of these TPUNs. This research combines numerical modeling and experimental characterization of TPUNs for SRM insulation. The TPUN thermophyscial properties and kinetic parameters will be characterized using thermogravimetric analysis, Multi-Function Sensor (MFS), and other thermal analyses. Numerical techniques for small scale physics from molecular dynamics (MD) simulations through population balance methods will be used to gain insight and intuition on the interactions between the polymeric and inorganic materials. These insights will help us to develop macroscopic kinetic models/descriptions in macroscale continuum models. These models will be first exercised against thermogravimetric and the MFS data, then small scale experiments using the LHMEL facility, and mesoscale experiments using AFRL Pi-K and Bates SRM firings. We formulated a simple non-charring ablation model, and then used it to perform a sensitivity analysis of failure time to four thermophysical properties. We found that failure time is most sensitive to the density and the heat of ablation, and is relatively insensitive to the thermal conductivity of the material. We reviewed numerical modeling of thermal protection materials literature, processed selective TPUNs, and calibrated a radiant heat apparatus to test TPUNs.

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Document Details

Document Type
Technical Report
Publication Date
Sep 30, 2006
Accession Number
ADA589776

Entities

People

  • J. H. Koo
  • O. D. Ezekoye

Organizations

  • University of Texas at Austin

Tags

Communities of Interest

  • Biomedical
  • Weapons Technologies

DTIC Thesaurus Topics

  • Ablative Materials
  • Composite Materials
  • Engineered Materials
  • Heat Transfer
  • Material Degradation Processes
  • Materials
  • Materials Laboratories
  • Materials Processing
  • Materials Science
  • Mechanical Engineering
  • Molecular Dynamics
  • Nanocomposites
  • Polymer-Matrix Nanocomposites
  • Resins
  • Rocket Engines
  • Thermal Conductivity
  • Thermophysical Properties

Readers

  • Computational Fluid Dynamics (CFD)
  • Rocket Propulsion.
  • Thermal Physics or Thermal Science.

Technology Areas

  • Microelectronics